Header menu link for other important links
X
Redox-Neutral Decarboxylative Cross-Coupling of Oxamates with Aryl Bromides
Akash Bisoyi, Vijay Simhadri Kumar, K. Surya, , Veera Yatham Reddy
Published in American Chemical Society
2023
Abstract
Dual nickel-photoredox-enabled direct synthesis of amides through cross-coupling of cesium oxamates with aryl bromides has been developed. This methodology’s key advantages are mild reaction conditions, utilizing organic dye as a photocatalyst, employing readily available starting chemicals as coupling partners and late-stage carbamoylation of pharmaceutically relevant molecules. DFT studies suggested that the nickel catalytic cycle proceeds via a radical addition pathway prior to the oxidative insertion. © 2023 The Authors. Published by American Chemical Society.
About the journal
JournalACS Organic and Inorganic Au
PublisherAmerican Chemical Society
ISSN2694247X